The Science

Super powerful quantum computing relies on quantum bits, aka qubits, which are the equivalent of the classical bits used in today’s computers. SQUIDs are being investigated for the development of qubits. However, system noise can destroy the data stored in the resulting qubits. Calculations have confirmed experimental evidence that oxygen molecules adsorbed on the surface of the SQUID are the most likely source of low-frequency magnetic noise. Scientists identified mitigation strategies, such as surface protection and improved vacuum environments. These approaches lowered the surface oxygen and the associated noise to levels needed for SQUIDs to be used in the next generation of computers.

The Impact

Superconducting devices are candidates for developing qubits. One type of device is called a SQUID for superconducting quantum interference device. It is based on a superconducting loop containing one or two Josephson junctions and allows measurement of quantized magnetic energy.  However, the ability to develop SQUID-based quantum computers will require the stored magnetic data survive for long times. Scientists discovered the origin of magnetic noise in these systems, and ways to minimize it. Their work provides a design strategy for the development of tunable superconducting qubits with long lifetimes.

Summary

In quantum computing, quantum information is lost due to a loss of synchronization (dephasing) in the electronic flow and energy relaxation. Magnetic flux noise is a dominant source of dephasing and energy relaxation in superconducting qubits. Recently reported experiments indicated that the detrimental noise is from unpaired magnetic defects on surfaces of superconducting devices. Theoretical predictions singled out oxygen as the cause of noise in these systems. In a team effort, theory calculations at the University of California, Irvine and experimental measurements by their collaborators showed that adsorbed molecular oxygen (O2 on the surfaces is the dominant contributor to magnetic noise for superconducting niobium and aluminum thin films. The mechanism is related to the outermost electrons of the oxygen molecule forming a magnetic spin-1 triplet state. Theory and experiment were iterated to find mitigation strategies. Surface treatment with ammonia and improving the sample vacuum environment dramatically reduced the surface contamination (to less than one oxygen molecule per 10 nm2), minimizing magnetic noise. In x-ray experiments at the Advanced Photon Source, scientists measured the suppression of magnetic spin and magnetic noise. Molecular oxygen was confirmed as the extrinsic noise source. The identification of this source explains the weak dependence of this type of noise on device materials. Also, discovering the origin of this noise invalidates prevailing theories for the noise based on defects at the metal-insulator interface. Suitable surface protection and improvements in the vacuum can lead to significant reductions in low-frequency magnetic noise. This new understanding of the origin of magnetic flux noise could lead to frequency-tunable superconducting qubits with improved dephasing times for practical quantum computers.

Funding

This work was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (density functional theory calculations), including use of the National Energy Research Scientific Computing Center and experimental research at the Advanced Photon Source, DOE Office of Science user facilities. This work was also supported by the U.S. Army Research Office, Google, and the Chinese National Science Foundation (Fudan University). Work at the National Institute of Standards and Technology was supported by the Laboratory for Physical Sciences, Army Research Office, and Defense Advanced Research Projects Agency.

Publications

P. Kumar, S. Sendelbach, M.A. Beck, J.W. Freeland, Z. Wang, H. Wang, C.C. Yu, R.Q. Wu, D.P. Pappas, and R. McDermott, "Origin and reduction of 1/f magnetic flux noise in superconducting devices." Physical Review Applied 6, 041001 (2016). [DOI: 10.1103/PhysRevApplied.6.041001]

H. Wang, C. Shi, J. Hu, S. Han, C.C. Yu, and R.Q. Wu, “Candidate source of flux noise in SQUIDs: Adsorbed oxygen molecules.” Physical Review Letters 115, 077002 (2015); Erratum Physical Review Letters 115, 249901 (2015). [DOI: 10.1103/PhysRevLett.115.077002]

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Journal Link: Physical Review Applied 6, 041001 (2016). [DOI: 10.1103/PhysRevApplied.6.041001]