Doe Science news source
The DOE Science News Source is a Newswise initiative to promote research news from the Office of Science of the DOE to the public and news media.
  • 2018-01-09 14:00:44
  • Article ID: 687623

Breaking Bad Metals with Neutrons

  • Credit: Argonne National Laboratory

    A comparison of the theoretical calculations (top row) and inelastic neutron scattering data from ARCS at the Spallation Neutron Source (bottom row) shows the excellent agreement between the two. The three figures represent different slices through the four-dimensional scattering volumes produced by the electronic excitations.

By exploiting the properties of neutrons to probe electrons in a metal, a team of researchers led by the U.S. Department of Energy’s (DOE) Argonne National Laboratory has gained new insight into the behavior of correlated electron systems, which are materials that have useful properties such as magnetism or superconductivity.

The research, to be published in Science, shows how well scientists can predict the properties and functionality of materials, allowing us to explore their potential to be used in novel ways.

“How do you get to a stage where the models are reliable? This
paper shows that we can now theoretically model even extremely
complex systems. These techniques could accelerate our discovery of new materials.” — Ray Osborn, Argonne senior scientist

“Our mission from the Department of Energy is to discover and then understand novel materials that could form the basis for completely new applications,” said lead author Ray Osborn, a senior scientist in Argonne’s Neutron and X-ray Scattering Group.

Osborn and his colleagues studied a strongly correlated electron system (CePd3) using neutron scattering to overcome the limitations of other techniques and reveal how the compound’s electrical properties change at high and low temperatures. Osborn expects the results to inspire similar research.

“Being able to predict with confidence the behavior of electrons as temperatures change should encourage a much more ambitious coupling of experimental results and models than has been previously attempted,” Osborn said.

“In many metals, we consider the mobile electrons responsible for electrical conduction as moving independently of each other, only weakly affected by electron-electron repulsion,” he said. “However, there is an important class of materials in which electron-electron interactions are so strong they cannot be ignored.”

Scientists have studied these strongly correlated electron systems for more than five decades, and one of the most important theoretical predictions is that at high temperatures the electron interactions cause random fluctuations that impede their mobility.

“They become ‘bad’ metals,” Osborn said. However, at low temperatures, the electronic excitations start to resemble those of normal metals, but with much-reduced electron velocities.

The existence of this crossover from incoherent random fluctuations at high temperature to coherent electronic states at low temperature had been postulated in 1985 by one of the co-authors, Jon Lawrence, a professor at the University of California, Irvine. Although there is some evidence for it in photoemission experiments, Argonne co-author Stephan Rosenkranz noted that it is very difficult to compare these measurements with realistic theoretical calculations because there are too many uncertainties in modeling the experimental intensities.

The team, based mainly at Argonne and other DOE laboratories, showed that neutrons probe the electrons in a different way that overcomes the limitations of photoemission spectroscopy and other techniques.

Making this work possible are advances in neutron spectroscopy at DOE’s Spallation Neutron Source (SNS) at Oak Ridge National Laboratory, a DOE Office of Science User Facility, and the United Kingdom’s ISIS Pulsed Neutron Source, which allow comprehensive measurements over a wide range of energies and momentum transfers. Both played critical roles in this study.

“Neutrons are absolutely essential for this research,” Osborn said. “Neutron scattering is the only technique that is sensitive to the whole spectrum of electronic fluctuations in four dimensions of momentum and energy, and the only technique that can be reliably compared to realistic theoretical calculations on an absolute intensity scale.”

With this study, these four-dimensional measurements have now been directly compared to calculations using new computational techniques specially developed for strongly correlated electron systems. The technique, known as Dynamical Mean Field Theory, defines a way of calculating electronic properties that include strong electron-electron interactions.

Osborn acknowledged the contributions of Eugene Goremychkin, a former Argonne scientist who led the data analysis, and Argonne theorist Hyowon Park, who performed the calculations. The agreement between theory and experiments was “truly remarkable,” Osborn said.

Looking ahead, researchers are optimistic about closing the gap between the results of condensed matter physics experiments and theoretical models.

“How do you get to a stage where the models are reliable?” Osborn said. “This paper shows that we can now theoretically model even extremely complex systems. These techniques could accelerate our discovery of new materials.”

Other Argonne authors of the paper, titled “Coherent Band Excitations in CePd3: A Comparison of Neutron Scattering and ab initio Theory,” are Park and John-Paul Castellan of the Materials Science Division. Also contributing to this work were researchers at the Joint Institute for Nuclear Research in Russia; the University of Illinois at Chicago; Karlsruhe Institute of Technology in Germany; Oak Ridge National Laboratory; Los Alamos National Laboratory and the University of California at Irvine.

Research at Argonne and Los Alamos was funded by DOE’s Materials Sciences and Engineering Division of the Office of Basic Energy Sciences. Research at Oak Ridge’s SNS was supported by the Scientific User Facilities Division of the Office of Basic Energy Sciences. Neutron experiments were performed at the SNS and the ISIS Pulsed Neutron Source, Rutherford Appleton Laboratory in the UK. Blues, a high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne, also contributed to this research.

Argonne National Laboratory seeks solutions to pressing national problems in science and technology. The nation's first national laboratory, Argonne conducts leading-edge basic and applied scientific research in virtually every scientific discipline. Argonne researchers work closely with researchers from hundreds of companies, universities, and federal, state and municipal agencies to help them solve their specific problems, advance America's scientific leadership and prepare the nation for a better future. With employees from more than 60 nations, Argonne is managed by UChicago Argonne, LLC for the U.S. Department of Energy's Office of Science.

The U.S. Department of Energy's Office of Science is the single largest supporter of basic research in the physical sciences in the United States and is working to address some of the most pressing challenges of our time. For more information, visit the Office of Science website.

  • Filters

  • × Clear Filters

Demonstrated Natural Refrigerant Replacements Could Reduce Energy Costs and Conserve the Environment

The 1987 Montreal Protocol and the 1997 Kyoto Protocol called for countries around the world to phase out substances that deplete the ozone layer and cause global warming, but many HVAC systems still use synthetic refrigerants that violate those international agreements and inflict environmental damage. Recently, Iranian researchers investigated how natural refrigerants could be used in geothermal heat pumps to reduce energy consumption and operating costs. They report their findings in the Journal of Renewable and Sustainable Energy.

The Behavior of Water: Scientists Find New Properties of H2O

A team of scientists has uncovered new molecular properties of water--a discovery of a phenomenon that had previously gone unnoticed.

Algorithm Provides Early Warning System for Tracking Groundwater Contamination

Scientists at the Department of Energy's Lawrence Berkeley National Laboratory (Berkeley Lab) and Savannah River National Laboratory have developed a low-cost method for real-time monitoring of pollutants using commonly available sensors.

Protons Get Zippier in Neutron-Rich Nuclei

A new study carried out at the Department of Energy's Thomas Jefferson National Accelerator Facility has confirmed that increasing the number of neutrons as compared to protons in the atom's nucleus also increases the average momentum of its protons. The nuclear physics result, which has implications for the dynamics of neutron stars, has been published in the journal Nature.

Sight Unseen: Novel Method Detects Evidence of Unmarked Human Graves

A new approach to find unmarked gravesites could help narrow the scope and potentially speed up the search for clues during crime scene investigations. Geospatial researchers with the Department of Energy's Oak Ridge National Laboratory and forensic scientists at University of Tennessee used LIDAR to detect telltale signs of recently buried human remains.

UT-ORNL team makes first particle accelerator beam measurement in six dimensions

The first full characterization measurement of an accelerator beam in six dimensions will advance the understanding and performance of current and planned accelerators around the world.

For UW Physicists, the 2-D Form of Tungsten Ditelluride Is Full of Surprises

In a paper published online July 23 in Nature, a UW-led research team reports that the 2-D form of tungsten ditelluride can undergo "ferroelectric switching" -- a first for a exfoliated 2-D material. Ferroelectric materials can have applications in memory storage, capacitors, RFID card technologies and even medical sensors.

Scientists Discover How to Protect Yeast From Damage in Biofuel Production

Some chemicals used to speed up the breakdown of plants for production of biofuels like ethanol are poison to the yeasts that turn the plant sugars into fuel. Researchers from the University of Wisconsin-Madison and several Department of Energy laboratories have identified two changes to a single gene that can make the yeast tolerate the pretreatment chemicals.

Lining Up the Surprising Behaviors of a Superconductor with One of the World's Strongest Magnets

Scientists have discovered that the electrical resistance of this material changes in an unusual way under very high magnetic fields--a finding that could help direct the search for materials that can perfectly conduct electricity at room temperature.

Hotter Temperatures Extend Growing Season for Peatland Plants

A study in Nature revealed that turning up the heat accelerates spring greening in vegetation and delays fall color change. The research team measured plant greenness over three years at the SPRUCE study, a unique ecosystem-scale experiment operated by DOE's Oak Ridge National Laboratory.

  • Filters

  • × Clear Filters

Four Argonne transportation and fuel experts collect Dept. of Energy honors

Four researchers at the U.S. Department of Energy's (DOE) Argonne National Laboratory have earned Distinguished Achievement awards for helping to reimagine transportation, sustainability and mobility.

From Hurricane Katrina Victim to Presidential Awardee: A SUNO Professor's Award-Winning Mentoring Efforts

Undergraduate students of Southern University at New Orleans (SUNO) biology professor Murty Kambhampati come to Brookhaven Lab during the summer to conduct research in natural resource management.

SNS completes full neutron production cycle at record power level

The Spallation Neutron Source at Oak Ridge National Laboratory has reached a new milestone by operating a complete neutron production run cycle at 1.3 megawatts. Achieving the record power level with a remarkable 94 percent accelerator beam availability establishes a new baseline of operation as well as a path to operate reliably at higher powers. Increased power offers researchers the ability to conduct faster scientific analyses using neutrons on more types of materials.

Milsmann earns prestigious NSF CAREER Award

Carsten Milsmann, assistant professor in the C. Eugene Bennett Department of Chemistry at West Virginia University, has earned the National Science Foundation's prestigious CAREER Award for research that could help develop solar energy applications that are more efficient and cheaper to produce.

46th annual SLAC Summer Institute celebrates Standard Model at 50

The event attracted 124 participants and explores the successes and challenges of the theory that describes subatomic particles and fundamental forces.

UW, PNNL to host energy research center focusing on bio-inspired design and assembly

The U.S. Department of Energy has awarded an expected $10.75 million, four-year grant to the University of Washington, the Pacific Northwest National Laboratory and other partner institutions for a new interdisciplinary research center to define the enigmatic rules governing how molecular-scale building blocks assemble into ordered structures & hierarchical materials.

Argonne among 10 recipients of competitive grant for ultrafast science

Argonne has been awarded U.S. Department of Energy funds to probe materials and chemical processes on time scales of a quadrillionth of a second or less.

One cool camera: LSST's cryostat assembly completed

Work on the camera for the future Large Synoptic Survey Telescope (LSST) has reached a major milestone with the completion and delivery of the camera's fully integrated cryostat. With 3.2 gigapixels, the LSST camera will be the largest digital camera ever built for ground-based astronomy. It's being assembled at the Department of Energy's SLAC National Accelerator Laboratory.

Risa Wechsler named director of KIPAC

Risa Wechsler has been appointed director of the Kavli Institute for Particle Astrophysics and Cosmology (KIPAC), a joint institute of the Department of Energy's SLAC National Accelerator Laboratory and Stanford University. On Sept. 15, she'll take over from Tom Abel, whose five-year term at the helm of the institute is coming to an end.

Ming Yi wins Spicer Award for superconductor research at SLAC's X-ray synchrotron

In recognition of her foundational superconductor research, Ming Yi has been awarded the 2018 William E. and Diane M. Spicer Young Investigator Award, which is presented to a young scientist who has made significant contributions to the Stanford Synchrotron Radiation Lightsource (SSRL) and the light source community. SSRL is a DOE Office of Science user facility at SLAC National Accelerator Laboratory.

  • Filters

  • × Clear Filters

Complex Networks Identify Genes for Biofuel Crops

Systems biology leads the way to exascale computing on Summit supercomputer.

Quantum Computing of an Atomic Nucleus

The first-ever computation of an atomic nucleus, the deuteron, on a quantum chip demonstrates that even today's rudimentary quantum computers can solve nuclear physics questions.

New Approach Yields High-Purity Radium for Medical Applications

Proton-irradiated thorium targets are successfully mined for therapeutic radium isotopes.

Steering Light with Dynamic Lens-on-MEMS

Scientists add active control to design capabilities for new lightweight flat optical devices.

Sugar-Coated Sheets Selectively Target Pathogens

Researchers design self-assembling nanosheets that mimic the surface of cells.

Tracking Down Helium-4's Quarks and Gluons

Scientists obtain the first exclusive measurement of deeply virtual Compton scattering of electrons off helium-4, vital to obtaining an unambiguous 3-D view of quarks and gluons within nuclei.

Predicting Magnetic Explosions: From Plasma Current Sheet Disruption to Fast Magnetic Reconnection

Supercomputer simulations and theoretical analysis shed new light on when and how fast reconnection occurs.

Is Nature Exclusively Left Handed? Using Chilled Atoms to Find Out

Elegant techniques of trapping and polarizing atoms open vistas for beta-decay tests of fundamental symmetries, key to understanding the most basic forces and particles constituting our universe.

As Future Batteries, Hybrid Supercapacitors Are Super-Charged

A new supercapacitor could be a competitive alternative to lithium-ion batteries.

Forever Young Catalyst Reduces Diesel Emissions

Atom probe tomography reveals key explanations for stable performance over a cutting-edge diesel-exhaust catalyst's lifetime.


Friday July 20, 2018, 03:00 PM

Department of Energy Invests $64 Million in Advanced Nuclear Technology

Rensselaer Polytechnic Institute (RPI)

Thursday July 19, 2018, 05:00 PM

Professor Miao Yu Named the Priti and Mukesh Chatter '82 Career Development Professor

Rensselaer Polytechnic Institute (RPI)

Tuesday July 03, 2018, 11:05 AM

2018 RHIC & AGS Annual Users' Meeting: 'Illuminating the QCD Landscape'

Brookhaven National Laboratory

Friday June 29, 2018, 06:05 PM

Argonne welcomes The Martian author Andy Weir

Argonne National Laboratory

Monday June 18, 2018, 09:55 AM

Creating STEM Knowledge and Innovations to Solve Global Issues Like Water, Food, and Energy

Illinois Mathematics and Science Academy (IMSA)

Friday June 15, 2018, 10:00 AM

Professor Emily Liu Receives $1.8 Million DoE Award for Solar Power Systems Research

Rensselaer Polytechnic Institute (RPI)

Thursday June 07, 2018, 03:05 PM

Celebrating 40 years of empowerment in science

Argonne National Laboratory

Monday May 07, 2018, 10:30 AM

Introducing Graduate Students Across the Globe to Photon Science

Brookhaven National Laboratory

Wednesday May 02, 2018, 04:05 PM

Students from Massachusetts and Washington Win DOE's 28th National Science Bowl(r)

Department of Energy, Office of Science

Thursday April 12, 2018, 07:05 PM

The Race for Young Scientific Minds

Argonne National Laboratory

Wednesday March 14, 2018, 02:05 PM

Q&A: Al Ashley Reflects on His Efforts to Diversify SLAC and Beyond

SLAC National Accelerator Laboratory

Thursday February 15, 2018, 12:05 PM

Insights on Innovation in Energy, Humanitarian Aid Highlight UVA Darden's Net Impact Week

University of Virginia Darden School of Business

Friday February 09, 2018, 11:05 AM

Ivy League Graduate, Writer and Activist with Dyslexia Visits CSUCI to Reframe the Concept of Learning Disabilities

California State University, Channel Islands

Wednesday January 17, 2018, 12:05 PM

Photographer Adam Nadel Selected as Fermilab's New Artist-in-Residence for 2018

Fermi National Accelerator Laboratory (Fermilab)

Wednesday January 17, 2018, 12:05 PM

Fermilab Computing Partners with Argonne, Local Schools for Hour of Code

Fermi National Accelerator Laboratory (Fermilab)

Wednesday December 20, 2017, 01:05 PM

Q&A: Sam Webb Teaches X-Ray Science from a Remote Classroom

SLAC National Accelerator Laboratory

Monday December 18, 2017, 01:05 PM

The Future of Today's Electric Power Systems

Rensselaer Polytechnic Institute (RPI)

Monday December 18, 2017, 12:05 PM

Supporting the Development of Offshore Wind Power Plants

Rensselaer Polytechnic Institute (RPI)

Tuesday October 03, 2017, 01:05 PM

Stairway to Science

Argonne National Laboratory

Thursday September 28, 2017, 12:05 PM

After-School Energy Rush

Argonne National Laboratory

Thursday September 28, 2017, 10:05 AM

Bringing Diversity Into Computational Science Through Student Outreach

Brookhaven National Laboratory

Thursday September 21, 2017, 03:05 PM

From Science to Finance: SLAC Summer Interns Forge New Paths in STEM

SLAC National Accelerator Laboratory

Thursday September 07, 2017, 02:05 PM

Students Discuss 'Cosmic Opportunities' at 45th Annual SLAC Summer Institute

SLAC National Accelerator Laboratory

Thursday August 31, 2017, 05:05 PM

Binghamton University Opens $70 Million Smart Energy Building

Binghamton University, State University of New York

Wednesday August 23, 2017, 05:05 PM

Widening Horizons for High Schoolers with Code

Argonne National Laboratory

Saturday May 20, 2017, 12:05 PM

Rensselaer Polytechnic Institute Graduates Urged to Embrace Change at 211th Commencement

Rensselaer Polytechnic Institute (RPI)

Monday May 15, 2017, 01:05 PM

ORNL, University of Tennessee Launch New Doctoral Program in Data Science

Oak Ridge National Laboratory

Friday April 07, 2017, 11:05 AM

Champions in Science: Profile of Jonathan Kirzner

Department of Energy, Office of Science

Wednesday April 05, 2017, 12:05 PM

High-Schooler Solves College-Level Security Puzzle From Argonne, Sparks Interest in Career

Argonne National Laboratory

Tuesday March 28, 2017, 12:05 PM

Champions in Science: Profile of Jenica Jacobi

Department of Energy, Office of Science

Friday March 24, 2017, 10:40 AM

Great Neck South High School Wins Regional Science Bowl at Brookhaven Lab

Brookhaven National Laboratory

Wednesday February 15, 2017, 04:05 PM

Middle Schoolers Test Their Knowledge at Science Bowl Competition

Argonne National Laboratory

Friday January 27, 2017, 04:00 PM

Haslam Visits ORNL to Highlight State's Role in Discovering Tennessine

Oak Ridge National Laboratory

Tuesday November 08, 2016, 12:05 PM

Internship Program Helps Foster Development of Future Nuclear Scientists

Oak Ridge National Laboratory

Friday May 13, 2016, 04:05 PM

More Than 12,000 Explore Jefferson Lab During April 30 Open House

Thomas Jefferson National Accelerator Facility

Monday April 25, 2016, 05:05 PM

Giving Back to National Science Bowl

Ames Laboratory

Friday March 25, 2016, 12:05 PM

NMSU Undergrad Tackles 3D Particle Scattering Animations After Receiving JSA Research Assistantship

Thomas Jefferson National Accelerator Facility

Tuesday February 02, 2016, 10:05 AM

Shannon Greco: A Self-Described "STEM Education Zealot"

Princeton Plasma Physics Laboratory

Monday November 16, 2015, 04:05 PM

Rare Earths for Life: An 85th Birthday Visit with Mr. Rare Earth

Ames Laboratory

Tuesday October 20, 2015, 01:05 PM

Meet Robert Palomino: 'Give Everything a Shot!'

Brookhaven National Laboratory

Tuesday April 22, 2014, 11:30 AM

University of Utah Makes Solar Accessible

University of Utah

Wednesday March 06, 2013, 03:40 PM

Student Innovator at Rensselaer Polytechnic Institute Seeks Brighter, Smarter, and More Efficient LEDs

Rensselaer Polytechnic Institute (RPI)

Friday November 16, 2012, 10:00 AM

Texas Tech Energy Commerce Students, Community Light up Tent City

Texas Tech University

Wednesday November 23, 2011, 10:45 AM

Don't Get 'Frosted' Over Heating Your Home This Winter

Temple University

Wednesday July 06, 2011, 06:00 PM

New Research Center To Tackle Critical Challenges Related to Aircraft Design, Wind Energy, Smart Buildings

Rensselaer Polytechnic Institute (RPI)

Friday April 22, 2011, 09:00 AM

First Polymer Solar-Thermal Device Heats Home, Saves Money

Wake Forest University

Showing results

0-4 Of 2215