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    The DOE Science News Source is a Newswise initiative to promote research news from the Office of Science of the DOE to the public and news media.
    • 2019-03-28 11:05:21
    • Article ID: 710351

    Synergy for Storage: Containing Nuclear Waste for Thousands of Years

    The diverse team at the WastePD Energy Frontier Research Center is learning the secrets of storage materials to contain Cold War leftovers.

    • Credit: Center for Performance and Design of Nuclear Waste Forms and Containers

      Researchers determined the structures that sometimes form where water (blue) and glass (gray) meet. These water-filled cavities can cause the glass to corrode suddenly.

    Browsing the Gilcrease Museum's collection of pre-Columbian American art and tools in Tulsa, OK, one keeps coming back to the obsidian knives, arrowheads (or "projectile points," to anthropologists), and even ear ornaments—glossy black, smooth, and glassy. For tens of thousands of years, indigenous peoples fashioned these items out of cooled lava, beautiful but also able to hold a keen edge for millennia. The same museum collection also features metal knives, some only a few centuries old, already pitted and rusted, and a range of ceramic items in varying stages of deterioration from surprisingly pristine to faded and cracked. Clearly, these different materials—glassy obsidian, earthy ceramic, and metallic—have properties that influence how they stand the test of time.

    "There are difficult issues in understanding how materials corrode over really long time spans," said Gerald Frankel, director of the Center for Performance and Design of Nuclear Waste Forms and Containers (WastePD). "These are scientific issues," he continued. "That's why we need fundamental science."

    Frankel, an Ohio State University professor, focuses that scientific lens on glass, ceramics, and metals used to trap Cold War leftovers, including ~90 million gallons of radioactive liquid and sludge (like wet beach sand). Solidifying the waste as glass or ceramics keeps it from leaking into soil and groundwater. The solid form holds the waste in for thousands of years, giving the radioactive matter time to decay to safer levels.

    To solidify the waste, it's prepared and mixed into the recipes for glass or ceramics. The solidified waste, a.k.a. waste form, is then set in specially designed metal canisters and stored. Defense-related waste in South Carolina is already being glassified. Another such plant is under construction in Washington State.

    Although glass, ceramics, and metal forms have been around for ages, researchers don't yet know key details about how materials crumble, dissolve, or otherwise come undone. "Right now, we don't understand waste form corrosion enough to come up with a good model," said Frankel.

    You can't just go off and do your thing alone. To develop the underlying science necessary to model waste form corrosion, Frankel brought together materials scientists, engineers, computer modelers, and theorists as WastePD, an Energy Frontier Research Center funded by the Department of Energy's (DOE's) Office of Science.

    The different perspectives give the team a broad view of scientific questions. Even better, they offer more techniques, tools, and know-how to get answers. But collaborating, especially across nine time zones, has its challenges. "We spend a lot of time interacting," said Frankel. "You can't just go off and do your thing alone."

    An early win for the team was solving a particularly vexing problem involving water on glass waste forms.

    Time and tide wait for no waste. Researchers assume that during the thousands of years that the waste rests in storage, rainwater or groundwater will get in.

    When glass is covered in water, either a protective or an unstable layer forms. The unstable film speeds glass corrosion, causing the glass to crumble far faster than if it had a protecting film.

    "To determine what drives the formation, we have to look at it in detail," said John Vienna, who leads WastePD's glass thrust area and works at DOE's Pacific Northwest National Laboratory.

    But the reactions occur underwater. While you could see the surface easily, conventional techniques aren't designed to get accurate data on an underwater surface. "It's been a Holy Grail of chemistry," said Vienna.

    The team found a way by collaborating. Each team member brought in ideas and applied them. It's like bringing together a dozen internationally renowned chefs and asking them to cook a fish, and then combining all that knowledge and techniques to do something nobody's seen before.

    They started by flash freezing pristine water on glass. It's like a frozen, frosted chocolate sheet cake with glass as the cake and water as the icing. They sliced a thin piece, like cutting a tiny serving, and analyzed it. They repeated the experiment every few seconds as the water caused an unstable porous layer to form on the glass, essentially creating a sophisticated flipbook.

    The troubling layer formed by the water and glass reacting scoops out tiny bits of glass from the surface and lets water get in, just as it could at a storage site. The film's structure—how many pores form, how deep, and how far apart—determines how fast the glass crumbles.

    The best is yet to be. "Our collaboration was something of a shotgun wedding at the start," said Vienna. The study of the glass corrosion in water is just one example of how bringing together different people, different instruments, and different ideas can lead a solution. "Now, we're making real progress by using techniques that were only used in one area and ways of looking at the problems."

    The Ohio State University leads WastePD, formed in 2016. It brings together scientists from Commissariat à l'Energie in France, Louisiana State University, Pacific Northwest National Laboratory, Pennsylvania State University, QuesTek Innovations LLC, Rensselaer Polytechnic Institute, University of North Texas, and University of Virginia. WastePD is one of 46 Energy Frontier Research Centers funded by the DOE's Office of Science. The centers mobilize the talents of experts and forge teams to lay the scientific groundwork to improve energy production and storage.

    This article is part of a series that explores how scientific teams come together in the Department of Energy's Energy Frontier Research Centers to solve intractable problems.

    The Office of Science is the single largest supporter of basic research in the physical sciences in the United States and is working to address some of the most pressing challenges of our time. For more information please visit https://science.energy.gov.

    Kristin Manke is a Communications Specialist on detail with the Office of Science, kristin.manke@science.doe.gov.

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    Blowing bubbles: PPPL scientist confirms novel way to launch and drive current in fusion plasmas

    Blowing bubbles: PPPL scientist confirms novel way to launch and drive current in fusion plasmas

    PPPL physicist Fatima Ebrahimi has used high-resolution computer simulations to confirm the practicality of the CHI start-up technique. The simulations show that CHI could produce electric current continuously in larger, more powerful tokamaks than exist today to produce stable fusion plasmas.

    A four-way switch promises greater tunability of layered materials

    A four-way switch promises greater tunability of layered materials

    A team from Oak Ridge National Laboratory and Vanderbilt University made the first experimental observation of a material phase that had been predicted but never seen.

    Scientists discover ​"ripple" in flexible material that could improve electronic properties

    Scientists discover ​"ripple" in flexible material that could improve electronic properties

    Argonne scientists have discovered an intriguing new behavior in a two-dimensional material at the atomic level as it is stretched and strained, like it would be in an actual flexible device.

    AI for Plant Breeding in an Ever-Changing Climate

    AI for Plant Breeding in an Ever-Changing Climate

    In this Q&A, Oak Ridge National Laboratory's Dan Jacobson talks about his team's work on a genomic selection algorithm, his vision for the future of environmental genomics, and the space where simulation meets AI.

    A New Parallel Strategy for Tackling Turbulence on Summit

    A New Parallel Strategy for Tackling Turbulence on Summit

    A team at Georgia Tech created a new turbulence algorithm optimized for the Summit supercomputer. It reached a performance of less than 15 seconds of wall-clock time per time step for more than 6 trillion grid points--a new world record surpassing the prior state of the art in the field for the size of the problem.

    Modeling Every Building in America Starts with Chattanooga

    Modeling Every Building in America Starts with Chattanooga

    An ORNL team used the Titan supercomputer to model every building serviced by the Electric Power Board of Chattanooga--all 178,368 of them--and discovered that EPB could potentially save $11-$35 million per year by adjusting electricity usage during peak critical times.

    Climate Change Expected to Shift Location of East Asian Monsoons

    Climate Change Expected to Shift Location of East Asian Monsoons

    More than a billion people in Asia depend on seasonal monsoons for their water needs. The Asian monsoon is closely linked to a planetary-scale tropical air flow which, according to a new study by Lawrence Berkeley National Laboratory, will most likely shift geographically as the climate continues to warm, resulting in less rainfall in certain regions.

    Nuclear warheads? This robot can find them

    Nuclear warheads? This robot can find them

    PPPL and Princeton University are developing a unique neutron-detector robot for arms control and nuclear security purposes. The robot recently passed a key neutron-detection test.

    Deep neural networks speed up weather and climate models

    Deep neural networks speed up weather and climate models

    A team of environmental and computation scientists at the U.S. Department of Energy's (DOE) Argonne National Laboratory are collaborating to use deep neural networks, a type of machine learning, to replace the parameterizations of certain physical schemes in the Weather Research and Forecasting Model, an extremely comprehensive model that simulates the evolution of many aspects of the physical world around us.

    New AI Model Tries to Synthesize Patient Data Like Doctors Do

    New AI Model Tries to Synthesize Patient Data Like Doctors Do

    A new approach developed by PNNL scientists improves the accuracy of patient diagnosis up to 20 percent when compared to other embedding approaches.


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    University of Maryland, Baltimore County wins DOE's 2019 CyberForce Competition(tm)

    University of Maryland, Baltimore County wins DOE's 2019 CyberForce Competition(tm)

    After a long suspenseful day, University of Maryland, Baltimore County earned the top spot as national winner of the U.S. Department of Energy's CyberForce Competition.

    In its 15th year, INCITE advances open science with supercomputer grants to 47 projects

    In its 15th year, INCITE advances open science with supercomputer grants to 47 projects

    The U.S. Department of Energy's Office of Science announced allocations of supercomputer access to 47 science projects for 2020--awarding 60 percent of the available time on some of the nation's most powerful supercomputers, with the ultimate goal of accelerating discovery and innovation. In 2020, 14 projects will run on Theta and 39 projects on Summit, where six of these projects will receive an allocation on both systems.

    ASU solar awards eclipse other universities in latest round of DOE funding

    ASU solar awards eclipse other universities in latest round of DOE funding

    ASU receives $9.8 million in Solar Energy Technologies Office Awards.

    DOE to Provide $10 Million for New Research into Ecosystem Processes

    The U.S. Department of Energy (DOE) announced a plan to provide $10 million for new observational and experimental studies aimed at improving the accuracy of today's Earth system models. Research will focus on three separate types of environments--terrestrial, watershed, and subsurface--where current models fall short of providing fully accurate representation.

    ORNL to host 13 teams for DOE CyberForce Competition

    ORNL to host 13 teams for DOE CyberForce Competition

    Oak Ridge National Laboratory will give college students the chance to practice cybersecurity skills in a real-world setting as a host of the Department of Energy's fifth collegiate CyberForce Competition on Nov. 16.

    Argonne nuclear engineer J'Tia Hart selected to Crain's Chicago Business "40 Under 40"

    Argonne nuclear engineer J'Tia Hart selected to Crain's Chicago Business "40 Under 40"

    Argonne nuclear engineer J'Tia Hart has been named to Crain's Chicago Business's "40 Under 40" list, which recognizes young leaders in a variety of fields.

    Lab-Wide Stormwater Capture, Transportation Savings and Clean-Up Efforts Win Federal Recognition

    Lab-Wide Stormwater Capture, Transportation Savings and Clean-Up Efforts Win Federal Recognition

    Argonne National Laboratory has won a regional Federal Green Challenge award for conserving resources and saving taxpayers' money.

    PPPL wins $70,000 in project funding from DOE for entrepreneurship

    PPPL wins $70,000 in project funding from DOE for entrepreneurship

    The Princeton Plasma Physics Laboratory receives funding from the U.S. Department of Energy for two projects to encourage entrepreneurship and mentor and encourage potential entrepreneurs.

    Brookhaven-Commonwealth Fusion Energy Project Wins DOE Funding

    Brookhaven-Commonwealth Fusion Energy Project Wins DOE Funding

    Brookhaven's Superconducting Magnet Division will partner with industry to develop and characterize superconducting power cables.

    U.S. Department of Energy to Hold Fifth CyberForce Competition(tm)

    U.S. Department of Energy to Hold Fifth CyberForce Competition(tm)

    Going on its fourth year, DOE's CyberForce Competition(tm) on Nov. 15-16 will give teams of cybersecurity students and professionals the opportunity to compete and refine their skills in real-time at 10 national laboratories across the U.S.


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    Harvesting Energy from Light using Bio-inspired Artificial Cells

    Harvesting Energy from Light using Bio-inspired Artificial Cells

    Scientists designed and connected two different artificial cells to each other to produce molecules called ATP (adenosine triphosphate).

    Engineering Living Scaffolds for Building Materials

    Engineering Living Scaffolds for Building Materials

    Bone and mollusk shells are composite systems that combine living cells and inorganic components. This allows them to regenerate and change structure while also being very strong and durable. Borrowing from this amazing complexity, researchers have been exploring a new class of materials called engineered living materials (ELMs).

    Excavating Quantum Information Buried in Noise

    Excavating Quantum Information Buried in Noise

    Researchers developed two new methods to assess and remove error in how scientists measure quantum systems. By reducing quantum "noise" - uncertainty inherent to quantum processes - these new methods improve accuracy and precision.

    How Electrons Move in a Catastrophe

    How Electrons Move in a Catastrophe

    Lanthanum strontium manganite (LSMO) is a widely applicable material, from magnetic tunnel junctions to solid oxide fuel cells. However, when it gets thin, its behavior changes for the worse. The reason why was not known. Now, using two theoretical methods, a team determined what happens.

    When Ions and Molecules Cluster

    When Ions and Molecules Cluster

    How an ion behaves when isolated within an analytical instrument can differ from how it behaves in the environment. Now, Xue-Bin Wang at Pacific Northwest National Laboratory devised a way to bring ions and molecules together in clusters to better discover their properties and predict their behavior.

    Tune in to Tetrahedral Superstructures

    Tune in to Tetrahedral Superstructures

    Shape affects how the particles fit together and, in turn, the resulting material. For the first time, a team observed the self-assembly of nanoparticles with tetrahedral shapes.

    Tracing Interstellar Dust Back to the Solar System's Formation

    Tracing Interstellar Dust Back to the Solar System's Formation

    This study is the first to confirm dust particles pre-dating the formation of our solar system. Further study of these materials will enable a deeper understanding of the processes that formed and have since altered them.

    Investigating Materials that Can Go the Distance in Fusion Reactors

    Investigating Materials that Can Go the Distance in Fusion Reactors

    Future fusion reactors will require materials that can withstand extreme operating conditions, including being bombarded by high-energy neutrons at high temperatures. Scientists recently irradiated titanium diboride (TiB2) in the High Flux Isotope Reactor (HFIR) to better understand the effects of fusion neutrons on performance.

    Better 3-D Imaging of Tumors in the Breast with Less Radiation

    Better 3-D Imaging of Tumors in the Breast with Less Radiation

    In breast cancer screening, an imaging technique based on nuclear medicine is currently being used as a successful secondary screening tool alongside mammography to improve the accuracy of the diagnosis. Now, a team is hoping to improve this imaging technique.

    Microbes are Metabolic Specialists

    Microbes are Metabolic Specialists

    Scientists can use genetic information to measure if microbes in the environment can perform specific ecological roles. Researchers recently analyzed the genomes of over 6,000 microbial species.


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