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    • 2019-03-28 11:05:21
    • Article ID: 710351

    Synergy for Storage: Containing Nuclear Waste for Thousands of Years

    The diverse team at the WastePD Energy Frontier Research Center is learning the secrets of storage materials to contain Cold War leftovers.

    • Credit: Center for Performance and Design of Nuclear Waste Forms and Containers

      Researchers determined the structures that sometimes form where water (blue) and glass (gray) meet. These water-filled cavities can cause the glass to corrode suddenly.

    Browsing the Gilcrease Museum's collection of pre-Columbian American art and tools in Tulsa, OK, one keeps coming back to the obsidian knives, arrowheads (or "projectile points," to anthropologists), and even ear ornaments—glossy black, smooth, and glassy. For tens of thousands of years, indigenous peoples fashioned these items out of cooled lava, beautiful but also able to hold a keen edge for millennia. The same museum collection also features metal knives, some only a few centuries old, already pitted and rusted, and a range of ceramic items in varying stages of deterioration from surprisingly pristine to faded and cracked. Clearly, these different materials—glassy obsidian, earthy ceramic, and metallic—have properties that influence how they stand the test of time.

    "There are difficult issues in understanding how materials corrode over really long time spans," said Gerald Frankel, director of the Center for Performance and Design of Nuclear Waste Forms and Containers (WastePD). "These are scientific issues," he continued. "That's why we need fundamental science."

    Frankel, an Ohio State University professor, focuses that scientific lens on glass, ceramics, and metals used to trap Cold War leftovers, including ~90 million gallons of radioactive liquid and sludge (like wet beach sand). Solidifying the waste as glass or ceramics keeps it from leaking into soil and groundwater. The solid form holds the waste in for thousands of years, giving the radioactive matter time to decay to safer levels.

    To solidify the waste, it's prepared and mixed into the recipes for glass or ceramics. The solidified waste, a.k.a. waste form, is then set in specially designed metal canisters and stored. Defense-related waste in South Carolina is already being glassified. Another such plant is under construction in Washington State.

    Although glass, ceramics, and metal forms have been around for ages, researchers don't yet know key details about how materials crumble, dissolve, or otherwise come undone. "Right now, we don't understand waste form corrosion enough to come up with a good model," said Frankel.

    You can't just go off and do your thing alone. To develop the underlying science necessary to model waste form corrosion, Frankel brought together materials scientists, engineers, computer modelers, and theorists as WastePD, an Energy Frontier Research Center funded by the Department of Energy's (DOE's) Office of Science.

    The different perspectives give the team a broad view of scientific questions. Even better, they offer more techniques, tools, and know-how to get answers. But collaborating, especially across nine time zones, has its challenges. "We spend a lot of time interacting," said Frankel. "You can't just go off and do your thing alone."

    An early win for the team was solving a particularly vexing problem involving water on glass waste forms.

    Time and tide wait for no waste. Researchers assume that during the thousands of years that the waste rests in storage, rainwater or groundwater will get in.

    When glass is covered in water, either a protective or an unstable layer forms. The unstable film speeds glass corrosion, causing the glass to crumble far faster than if it had a protecting film.

    "To determine what drives the formation, we have to look at it in detail," said John Vienna, who leads WastePD's glass thrust area and works at DOE's Pacific Northwest National Laboratory.

    But the reactions occur underwater. While you could see the surface easily, conventional techniques aren't designed to get accurate data on an underwater surface. "It's been a Holy Grail of chemistry," said Vienna.

    The team found a way by collaborating. Each team member brought in ideas and applied them. It's like bringing together a dozen internationally renowned chefs and asking them to cook a fish, and then combining all that knowledge and techniques to do something nobody's seen before.

    They started by flash freezing pristine water on glass. It's like a frozen, frosted chocolate sheet cake with glass as the cake and water as the icing. They sliced a thin piece, like cutting a tiny serving, and analyzed it. They repeated the experiment every few seconds as the water caused an unstable porous layer to form on the glass, essentially creating a sophisticated flipbook.

    The troubling layer formed by the water and glass reacting scoops out tiny bits of glass from the surface and lets water get in, just as it could at a storage site. The film's structure—how many pores form, how deep, and how far apart—determines how fast the glass crumbles.

    The best is yet to be. "Our collaboration was something of a shotgun wedding at the start," said Vienna. The study of the glass corrosion in water is just one example of how bringing together different people, different instruments, and different ideas can lead a solution. "Now, we're making real progress by using techniques that were only used in one area and ways of looking at the problems."

    The Ohio State University leads WastePD, formed in 2016. It brings together scientists from Commissariat à l'Energie in France, Louisiana State University, Pacific Northwest National Laboratory, Pennsylvania State University, QuesTek Innovations LLC, Rensselaer Polytechnic Institute, University of North Texas, and University of Virginia. WastePD is one of 46 Energy Frontier Research Centers funded by the DOE's Office of Science. The centers mobilize the talents of experts and forge teams to lay the scientific groundwork to improve energy production and storage.

    This article is part of a series that explores how scientific teams come together in the Department of Energy's Energy Frontier Research Centers to solve intractable problems.

    The Office of Science is the single largest supporter of basic research in the physical sciences in the United States and is working to address some of the most pressing challenges of our time. For more information please visit https://science.energy.gov.

    Kristin Manke is a Communications Specialist on detail with the Office of Science, kristin.manke@science.doe.gov.

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    Chemistry finding could make solar energy more efficient

    Chemistry finding could make solar energy more efficient

    Scientists for the first time have developed a single molecule that can absorb sunlight efficiently and also act as a catalyst to transform solar energy into hydrogen, a clean alternative to fuel for things like gas-powered vehicles. This new molecule collects energy from the entire visible spectrum, and can harness more than 50% more solar energy than current solar cells can. The finding could help humans transition away from fossil fuels and toward energy sources that do not contribute to climate change.

    New model helps pave the way to bringing clean fusion energy down to Earth

    New model helps pave the way to bringing clean fusion energy down to Earth

    State-of-the-art simulation confirms a key source of heat and energy loss in spherical fusion facilities.

    Rising global temperatures turn northern permafrost region into significant carbon source

    Rising global temperatures turn northern permafrost region into significant carbon source

    A new study that incorporates datasets gathered from more than 100 sites by institutions including the U.S. Department of Energy's (DOE) Argonne National Laboratory, suggests that decomposition of organic matter in permafrost soil is substantially larger than previously thought, demonstrating the significant impact that emissions from the permafrost soil could have on the greenhouse effect and global warming.

    Transformative 'Green' Accelerator Achieves World's First 8-pass Full Energy Recovery

    Transformative 'Green' Accelerator Achieves World's First 8-pass Full Energy Recovery

    Scientists from Cornell University and Brookhaven National Laboratory (BNL) have successfully demonstrated the world's first capture and reuse of energy in a multi-turn particle accelerator, where electrons are accelerated and decelerated in multiple stages and transported at different energies through a single beamline.

    First detailed electronic study of new nickelate superconductor finds 3D metallic state

    First detailed electronic study of new nickelate superconductor finds 3D metallic state

    It represents an entirely new type of ground state for transition metal oxides, and opens new directions for experiments and theoretical studies of how superconductivity arises and how it can be optimized in this system and possibly in other compounds.

    What's MER? It's a Way to Measure Quantum Materials, and It's Telling US New and Interesting Things

    What's MER? It's a Way to Measure Quantum Materials, and It's Telling US New and Interesting Things

    Experimental physicists have combined several measurements of quantum materials into one in their ongoing quest to learn more about manipulating and controlling the behavior of them for possible applications. They even coined a term for it-- Magneto-elastoresistance, or MER.

    Scientists pioneer new generation of semiconductor neutron detector

    Scientists pioneer new generation of semiconductor neutron detector

    In a new study, scientists have developed a new type of semiconductor neutron detector that boosts detection rates by reducing the number of steps involved in neutron capture and transduction.

    Connecting the dots in the sky could shed new light on dark matter

    Connecting the dots in the sky could shed new light on dark matter

    Astrophysicists have come a step closer to understanding the origin of a faint glow of gamma rays covering the night sky. They found that this light is brighter in regions that contain a lot of matter and dimmer where matter is sparser - a correlation that could help them narrow down the properties of exotic astrophysical objects and invisible dark matter.

    Nano-objects of Desire: Assembling Ordered Nanostructures in 3-D

    Nano-objects of Desire: Assembling Ordered Nanostructures in 3-D

    A new DNA-programmable nanofabrication platform organizes inorganic or biological nanocomponents in the same prescribed ways.

    New computer code could reach fusion faster

    New computer code could reach fusion faster

    Scientists often make progress by coming up with new ways to look at old problems. That has happened at PPPL, where physicists have used a simple insight to capture the complex effects of many high-frequency waves in a fusion plasma.


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    Team led by PPPL wins major supercomputer time to help capture on Earth the fusion that powers the sun and stars

    Team led by PPPL wins major supercomputer time to help capture on Earth the fusion that powers the sun and stars

    PPPL will use INCITE-award time on Summit and Theta supercomputers to develop predictions for the performance of ITER, the international experiment under construction to demonstrate the feasibility of fusion energy.

    Department of Energy Announces $625 Million for New Quantum Centers

    The U.S. Department of Energy (DOE) announced up to $625 million over the next five years to establish two to five multidisciplinary Quantum Information Science (QIS) Research Centers in support of the National Quantum Initiative.

    Department of Energy to Provide $75 Million for Bioenergy Crops Research

    The U.S. Department of Energy (DOE) announced a plan to provide up to $75 million over five years for research to develop sustainable bioenergy crops tolerant of environmental stress and resilient to changing environmental conditions.

    Jefferson Lab to be Major Partner in Electron Ion Collider Project

    Jefferson Lab to be Major Partner in Electron Ion Collider Project

    The Department of Energy announced that it has taken the next step toward construction of an Electron Ion Collider (EIC) in the United States. DOE announced on Thursday that the collider will be sited at DOE's Brookhaven National Laboratory in Upton, N.Y. In addition, DOE's Thomas Jefferson National Accelerator Facility will be a major partner in realizing the EIC, providing key support to build this next new collider, which will be the most advanced particle collider of its type ever built.

    Department of Energy Selects Site for Electron-Ion Collider

    Department of Energy Selects Site for Electron-Ion Collider

    UPTON, NY-- Yesterday, the U.S. Department of Energy (DOE) named Brookhaven National Laboratory on Long Island in New York as the site for building an Electron-Ion Collider (EIC), a one-of-a-kind nuclear physics research facility. This announcement, following DOE's approval of "mission need" (known as Critical Decision 0) on December 19, 2019, enables work to begin on R&D and the conceptual design for this next-generation collider at Brookhaven Lab.

    Department of Energy Announces $32 Million for Small Business Research and Development Grants

    U.S. Secretary of Energy Dan Brouillette announced that the Department of Energy (DOE) will award 158 grants totaling $32 million to 118 small businesses in 32 states. Funded through DOE's Small Business Innovation Research (SBIR) and Small Business Technology Transfer (STTR) programs, these selections are for Phase I research and development.

    Summit Charts a Course to Uncover the Origins of Genetic Diseases

    Summit Charts a Course to Uncover the Origins of Genetic Diseases

    Gene mutations can interfere with how the body expresses genes and cause disease. To better understand this connection, researchers recently developed a model of the transcription preinitiation complex (PIC).

    Alex Nagy, a "creative and energetic" engineer, is named a Distinguished Engineering Fellow

    Alex Nagy, a "creative and energetic" engineer, is named a Distinguished Engineering Fellow

    Feature profiles PPPL Distinguished Engineering Fellow recipient Alex Nagy

    PPPL honors physicists Igor Kaganovich and Yevgeny Raitses with Kaul Foundation Prize

    PPPL honors physicists Igor Kaganovich and Yevgeny Raitses with Kaul Foundation Prize

    Profiles of winners of PPPL's 2019 Kaul Foundation Prize recipients.

    The Quantum Information Edge Launches to Accelerate Quantum Computing R&D for Breakthrough Science

    The Quantum Information Edge Launches to Accelerate Quantum Computing R&D for Breakthrough Science

    A nationwide alliance of national labs, universities, and industry launched today to advance the frontiers of quantum computing systems designed to solve urgent scientific challenges and maintain U.S. leadership in next-generation information technology. The Quantum Information Edge strategic alliance is led by Lawrence Berkeley National Laboratory (Berkeley Lab) and Sandia National Laboratories.


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    Harvesting Energy from Light using Bio-inspired Artificial Cells

    Harvesting Energy from Light using Bio-inspired Artificial Cells

    Scientists designed and connected two different artificial cells to each other to produce molecules called ATP (adenosine triphosphate).

    Engineering Living Scaffolds for Building Materials

    Engineering Living Scaffolds for Building Materials

    Bone and mollusk shells are composite systems that combine living cells and inorganic components. This allows them to regenerate and change structure while also being very strong and durable. Borrowing from this amazing complexity, researchers have been exploring a new class of materials called engineered living materials (ELMs).

    Excavating Quantum Information Buried in Noise

    Excavating Quantum Information Buried in Noise

    Researchers developed two new methods to assess and remove error in how scientists measure quantum systems. By reducing quantum "noise" - uncertainty inherent to quantum processes - these new methods improve accuracy and precision.

    How Electrons Move in a Catastrophe

    How Electrons Move in a Catastrophe

    Lanthanum strontium manganite (LSMO) is a widely applicable material, from magnetic tunnel junctions to solid oxide fuel cells. However, when it gets thin, its behavior changes for the worse. The reason why was not known. Now, using two theoretical methods, a team determined what happens.

    When Ions and Molecules Cluster

    When Ions and Molecules Cluster

    How an ion behaves when isolated within an analytical instrument can differ from how it behaves in the environment. Now, Xue-Bin Wang at Pacific Northwest National Laboratory devised a way to bring ions and molecules together in clusters to better discover their properties and predict their behavior.

    Tune in to Tetrahedral Superstructures

    Tune in to Tetrahedral Superstructures

    Shape affects how the particles fit together and, in turn, the resulting material. For the first time, a team observed the self-assembly of nanoparticles with tetrahedral shapes.

    Tracing Interstellar Dust Back to the Solar System's Formation

    Tracing Interstellar Dust Back to the Solar System's Formation

    This study is the first to confirm dust particles pre-dating the formation of our solar system. Further study of these materials will enable a deeper understanding of the processes that formed and have since altered them.

    Investigating Materials that Can Go the Distance in Fusion Reactors

    Investigating Materials that Can Go the Distance in Fusion Reactors

    Future fusion reactors will require materials that can withstand extreme operating conditions, including being bombarded by high-energy neutrons at high temperatures. Scientists recently irradiated titanium diboride (TiB2) in the High Flux Isotope Reactor (HFIR) to better understand the effects of fusion neutrons on performance.

    Better 3-D Imaging of Tumors in the Breast with Less Radiation

    Better 3-D Imaging of Tumors in the Breast with Less Radiation

    In breast cancer screening, an imaging technique based on nuclear medicine is currently being used as a successful secondary screening tool alongside mammography to improve the accuracy of the diagnosis. Now, a team is hoping to improve this imaging technique.

    Microbes are Metabolic Specialists

    Microbes are Metabolic Specialists

    Scientists can use genetic information to measure if microbes in the environment can perform specific ecological roles. Researchers recently analyzed the genomes of over 6,000 microbial species.


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