The DOE Science News Source is a Newswise initiative to promote research news from the Office of Science of the DOE to the public and news media.
Oak Ridge National Laboratory

Pure promethium: ORNL extracts in-demand isotope from plutonium leftovers

10-Mar-2021 5:05 PM EST, by Oak Ridge National Laboratory

Newswise — A new method developed at Oak Ridge National Laboratory proves one effort’s trash is another’s valuable isotope.

One of the byproducts of the Department of Energy lab’s national plutonium-238 production program is promethium-147, a rare isotope used in nuclear batteries and to measure the thickness of materials.

It’s difficult and costly to dispose of waste containing radioactive elements left over after neptunium-237 targets are irradiated in the High Flux Isotope Reactor, a DOE Office of Science user facility, to produce Pu-238 for space exploration. But last year, a new ORNL project for the DOE Isotope Program began mining Pm-147 from the fission products left when Pu-238 is separated out of the target.

This effort‘s primary goal is to reestablish domestic production of Pm-147, which is in short supply, and it has a side benefit: reducing the concentrations of radioactive elements in the waste, so that it can be disposed of safely in simpler, less expensive ways both now and in the future.

“In the process of recovering a valuable product that the DOE Isotope Program wants, we realized we can reduce our disposal costs,” said ORNL’s Richard Mayes, group leader for Emerging Isotope Research. “There’s some synergy.”

Pm-147 isn’t the only valuable metal in the Pu-238 production waste stream that is of interest to the DOE Isotope Program, but it’s the first Mayes’ team has successfully extracted. ORNL’s Susan Hogle wrote the original proposal to mine Pm-147 from Pu-238 waste and provides computational support detailing potential isotopes present in the solution, and Mayes has been working with Lætitia Delmau, interim group leader for Radiochemical Separations Science Group at ORNL, to develop a process to extract and purify it.

“Currently, we’re the only producers of Pm-147 in the U.S., and there’s a market for it,” Mayes said. Research indicates it could have additional applications in medical imaging and as a radioisotope to generate power for space probes.

While the Pu-238 Supply Program is funded by NASA and managed through DOE’s Office of Nuclear Energy, the recovery of Pm-147 is funded by the DOE Isotope Program within DOE’s Office of Science.

ORNL is also pursuing research for the DOE Isotope Program in which neodymium-146 is irradiated in the High Flux Isotope Reactor, or HFIR to make Pm-147. This process would provide a new alternative, strengthening the domestic supply chain for this important isotope, and mitigating U.S. dependency on a single foreign supply.

Mayes’ team’s efforts are tied to the Pu-238 production schedule, which is currently between two and four processing cycles a year. They estimate that there are roughly hundreds of curies of Pm-147 in each batch. Working in around-the-clock shifts for several days, the team uses hot cells in ORNL’s Radiochemical Engineering Development Center, or REDC, to isolate a concentrated batch of Pm-147 from the solution of Pu-238 byproducts.

That batch is then transferred into a shielded cave —a smaller type of hot cell — at the REDC, where it’s purified and readied to ship to DOE Isotope Program customers. The process involves a few months of effort and around 20 people.

The team will spend the next year demonstrating whether the recovery of Pm-147 from Pu-238 byproducts is sustainable. If so, the project should grow alongside the Pu-238 program. The lab’s goal is to produce enough Pu-238 to yield 1.5 kilograms annually of plutonium oxide, to meet NASA’s demands for deep space travel. ORNL-produced plutonium oxide is on board the Perseverance rover now exploring Mars.

Delmau, who specializes in radiochemical separations, said Pm-147 is one of about a dozen elements left after processing Pu-238, and isolating individual elements takes work.

“The separation of lanthanides from each other and from trivalent actinides has been a challenge for decades,” she said. “When elements have the same chemical properties, it can be very difficult to pick one out.”

At the moment, Pm-147 is the only isotope being harvested from the waste stream, but an important side benefit of the project ultimately could be a substantial decrease in the amount of transuranic material the lab must dispose of. Mayes said successful efforts with Pm-147 may lead to the extraction of other materials at ORNL.

“We have a waste stream that has valuable products in it — products that could have many uses,” he said. “Our national labs have the resources and experience to safely and efficiently isolate them.”

UT-Battelle manages ORNL for the Department of Energy’s Office of Science, the single largest supporter of basic research in the physical sciences in the United States. The Office of Science is working to address some of the most pressing challenges of our time. For more information, please visit energy.gov/science.

 

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Newswise:Video Embedded ornl-partners-on-science-kits-for-stem-schools
VIDEO
Released: 17-May-2021 5:05 PM EDT
ORNL partners on science kits for STEM schools
Oak Ridge National Laboratory

Oak Ridge National Laboratory, the U.S. Department of Energy, the Center of Science and Industry and the Tennessee STEM Innovation Network have partnered to deliver hundreds of free science kits called Learning Lunchboxes to STEM-designated schools in East Tennessee.

Newswise: Argonne senior chemist Robert Tranter named fellow of the Combustion Institute
Released: 17-May-2021 11:40 AM EDT
Argonne senior chemist Robert Tranter named fellow of the Combustion Institute
Argonne National Laboratory

Argonne senior chemist Robert Tranter, a shockwave chemist, was named a fellow of the Combustion Institute.

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Released: 14-May-2021 4:05 PM EDT
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Newswise: Not Just Disturbance: Turbulence Protects Fusion Reactor Walls
Released: 14-May-2021 4:05 PM EDT
Not Just Disturbance: Turbulence Protects Fusion Reactor Walls
Department of Energy, Office of Science

To operate successfully, ITER and future fusion energy reactors cannot allow melting of the walls of the divertor plates that remove excess heat from the plasma in a reactor. These walls are especially at risk of melting when heat is applied to narrow areas. Now, however, an extreme-scale computing analysis indicates that turbulence will reduce that risk.

Newswise: Enhancing Land Surface Models to Grow Perennial Bioenergy Crops
Released: 14-May-2021 3:35 PM EDT
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To understand the effects of expanding biofuel production, scientists must accurately represent biofuel crops in land surface models. Using observations from biofuel plants in the Midwestern United States, researchers simulated two biofuel perennial plants, miscanthus and switchgrass. The simulations indicate these high-yield perennial crops have several advantages over traditional annual bioenergy crops—they assimilate more carbon dioxide, and they require fewer nutrients and less water.

Newswise: Enhancing Land Surface Models to Grow Perennial Bioenergy Crops
Released: 14-May-2021 3:35 PM EDT
Enhancing Land Surface Models to Grow Perennial Bioenergy Crops
Department of Energy, Office of Science

To understand the effects of expanding biofuel production, scientists must accurately represent biofuel crops in land surface models. Using observations from biofuel plants in the Midwestern United States, researchers simulated two biofuel perennial plants, miscanthus and switchgrass. The simulations indicate these high-yield perennial crops have several advantages over traditional annual bioenergy crops—they assimilate more carbon dioxide, and they require fewer nutrients and less water.

Newswise: Harvesting Light Like Nature Does
Released: 14-May-2021 2:55 PM EDT
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Newswise: 050721-ber-earths-atomosphere.jpg?itok=-W-tcpvH
Released: 14-May-2021 2:50 PM EDT
Scientists Check the Math for Improved Models of Liquids and Gases in Earth’s Atmosphere
Department of Energy, Office of Science

Discretization is the process of converting continuous models and variables, such as wind speed, into discrete versions to make equations that are compatible with computer analysis. Energy consistent discretization ensures that the method does not have any inaccurate sources of energy that can lead to unstable and unrealistic simulations. In this research, scientists provided a discretization for equations used by global models of the Earth’s atmosphere.

View More
Newswise:Video Embedded ornl-partners-on-science-kits-for-stem-schools
VIDEO
Released: 17-May-2021 5:05 PM EDT
ORNL partners on science kits for STEM schools
Oak Ridge National Laboratory

Oak Ridge National Laboratory, the U.S. Department of Energy, the Center of Science and Industry and the Tennessee STEM Innovation Network have partnered to deliver hundreds of free science kits called Learning Lunchboxes to STEM-designated schools in East Tennessee.

Newswise: Argonne senior chemist Robert Tranter named fellow of the Combustion Institute
Released: 17-May-2021 11:40 AM EDT
Argonne senior chemist Robert Tranter named fellow of the Combustion Institute
Argonne National Laboratory

Argonne senior chemist Robert Tranter, a shockwave chemist, was named a fellow of the Combustion Institute.

Newswise:Video Embedded successful-start-of-dark-energy-spectroscopic-instrument-desi-follows-record-setting-trial-run
VIDEO
Released: 17-May-2021 9:00 AM EDT
Successful Start of Dark Energy Spectroscopic Instrument (DESI) Follows Record-Setting Trial Run
Lawrence Berkeley National Laboratory

A five-year quest to map the universe and unravel the mysteries of “dark energy” is beginning officially today, May 17, at Kitt Peak National Observatory near Tucson, Arizona. To complete its quest, the Dark Energy Spectroscopic Instrument (DESI) will capture and study the light from tens of millions of galaxies and other distant objects in the universe.

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Released: 14-May-2021 5:20 PM EDT
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PNNL researchers developed an innovative capability to rapidly separate, monitor, and tightly control specific uranium and plutonium ratios in real-time—an important achievement in efficiently controlling the resulting product and safeguarding nuclear material.

Newswise: Not Just Disturbance: Turbulence Protects Fusion Reactor Walls
Released: 14-May-2021 4:05 PM EDT
Not Just Disturbance: Turbulence Protects Fusion Reactor Walls
Department of Energy, Office of Science

To operate successfully, ITER and future fusion energy reactors cannot allow melting of the walls of the divertor plates that remove excess heat from the plasma in a reactor. These walls are especially at risk of melting when heat is applied to narrow areas. Now, however, an extreme-scale computing analysis indicates that turbulence will reduce that risk.

Newswise: Not Just Disturbance: Turbulence Protects Fusion Reactor Walls
Released: 14-May-2021 4:05 PM EDT
Not Just Disturbance: Turbulence Protects Fusion Reactor Walls
Department of Energy, Office of Science

To operate successfully, ITER and future fusion energy reactors cannot allow melting of the walls of the divertor plates that remove excess heat from the plasma in a reactor. These walls are especially at risk of melting when heat is applied to narrow areas. Now, however, an extreme-scale computing analysis indicates that turbulence will reduce that risk.

Newswise: Enhancing Land Surface Models to Grow Perennial Bioenergy Crops
Released: 14-May-2021 3:35 PM EDT
Enhancing Land Surface Models to Grow Perennial Bioenergy Crops
Department of Energy, Office of Science

To understand the effects of expanding biofuel production, scientists must accurately represent biofuel crops in land surface models. Using observations from biofuel plants in the Midwestern United States, researchers simulated two biofuel perennial plants, miscanthus and switchgrass. The simulations indicate these high-yield perennial crops have several advantages over traditional annual bioenergy crops—they assimilate more carbon dioxide, and they require fewer nutrients and less water.

Newswise: Enhancing Land Surface Models to Grow Perennial Bioenergy Crops
Released: 14-May-2021 3:35 PM EDT
Enhancing Land Surface Models to Grow Perennial Bioenergy Crops
Department of Energy, Office of Science

To understand the effects of expanding biofuel production, scientists must accurately represent biofuel crops in land surface models. Using observations from biofuel plants in the Midwestern United States, researchers simulated two biofuel perennial plants, miscanthus and switchgrass. The simulations indicate these high-yield perennial crops have several advantages over traditional annual bioenergy crops—they assimilate more carbon dioxide, and they require fewer nutrients and less water.

Newswise: Harvesting Light Like Nature Does
Released: 14-May-2021 2:55 PM EDT
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A new class of bio-inspired two-dimensional (2D) hybrid nanomaterials mimic the ability of photosynthetic plants and bacteria.

Newswise: 050721-ber-earths-atomosphere.jpg?itok=-W-tcpvH
Released: 14-May-2021 2:50 PM EDT
Scientists Check the Math for Improved Models of Liquids and Gases in Earth’s Atmosphere
Department of Energy, Office of Science

Discretization is the process of converting continuous models and variables, such as wind speed, into discrete versions to make equations that are compatible with computer analysis. Energy consistent discretization ensures that the method does not have any inaccurate sources of energy that can lead to unstable and unrealistic simulations. In this research, scientists provided a discretization for equations used by global models of the Earth’s atmosphere.

View More
Newswise:Video Embedded ornl-partners-on-science-kits-for-stem-schools
VIDEO
Released: 17-May-2021 5:05 PM EDT
ORNL partners on science kits for STEM schools
Oak Ridge National Laboratory

Oak Ridge National Laboratory, the U.S. Department of Energy, the Center of Science and Industry and the Tennessee STEM Innovation Network have partnered to deliver hundreds of free science kits called Learning Lunchboxes to STEM-designated schools in East Tennessee.

Newswise: Argonne senior chemist Robert Tranter named fellow of the Combustion Institute
Released: 17-May-2021 11:40 AM EDT
Argonne senior chemist Robert Tranter named fellow of the Combustion Institute
Argonne National Laboratory

Argonne senior chemist Robert Tranter, a shockwave chemist, was named a fellow of the Combustion Institute.

Newswise:Video Embedded successful-start-of-dark-energy-spectroscopic-instrument-desi-follows-record-setting-trial-run
VIDEO
Released: 17-May-2021 9:00 AM EDT
Successful Start of Dark Energy Spectroscopic Instrument (DESI) Follows Record-Setting Trial Run
Lawrence Berkeley National Laboratory

A five-year quest to map the universe and unravel the mysteries of “dark energy” is beginning officially today, May 17, at Kitt Peak National Observatory near Tucson, Arizona. To complete its quest, the Dark Energy Spectroscopic Instrument (DESI) will capture and study the light from tens of millions of galaxies and other distant objects in the universe.

Newswise: Recycling Gives New Purpose to Spent Nuclear Fuel
Released: 14-May-2021 5:20 PM EDT
Recycling Gives New Purpose to Spent Nuclear Fuel
Pacific Northwest National Laboratory

PNNL researchers developed an innovative capability to rapidly separate, monitor, and tightly control specific uranium and plutonium ratios in real-time—an important achievement in efficiently controlling the resulting product and safeguarding nuclear material.

Newswise: Not Just Disturbance: Turbulence Protects Fusion Reactor Walls
Released: 14-May-2021 4:05 PM EDT
Not Just Disturbance: Turbulence Protects Fusion Reactor Walls
Department of Energy, Office of Science

To operate successfully, ITER and future fusion energy reactors cannot allow melting of the walls of the divertor plates that remove excess heat from the plasma in a reactor. These walls are especially at risk of melting when heat is applied to narrow areas. Now, however, an extreme-scale computing analysis indicates that turbulence will reduce that risk.

Newswise: Not Just Disturbance: Turbulence Protects Fusion Reactor Walls
Released: 14-May-2021 4:05 PM EDT
Not Just Disturbance: Turbulence Protects Fusion Reactor Walls
Department of Energy, Office of Science

To operate successfully, ITER and future fusion energy reactors cannot allow melting of the walls of the divertor plates that remove excess heat from the plasma in a reactor. These walls are especially at risk of melting when heat is applied to narrow areas. Now, however, an extreme-scale computing analysis indicates that turbulence will reduce that risk.

Newswise: Enhancing Land Surface Models to Grow Perennial Bioenergy Crops
Released: 14-May-2021 3:35 PM EDT
Enhancing Land Surface Models to Grow Perennial Bioenergy Crops
Department of Energy, Office of Science

To understand the effects of expanding biofuel production, scientists must accurately represent biofuel crops in land surface models. Using observations from biofuel plants in the Midwestern United States, researchers simulated two biofuel perennial plants, miscanthus and switchgrass. The simulations indicate these high-yield perennial crops have several advantages over traditional annual bioenergy crops—they assimilate more carbon dioxide, and they require fewer nutrients and less water.

Newswise: Enhancing Land Surface Models to Grow Perennial Bioenergy Crops
Released: 14-May-2021 3:35 PM EDT
Enhancing Land Surface Models to Grow Perennial Bioenergy Crops
Department of Energy, Office of Science

To understand the effects of expanding biofuel production, scientists must accurately represent biofuel crops in land surface models. Using observations from biofuel plants in the Midwestern United States, researchers simulated two biofuel perennial plants, miscanthus and switchgrass. The simulations indicate these high-yield perennial crops have several advantages over traditional annual bioenergy crops—they assimilate more carbon dioxide, and they require fewer nutrients and less water.

Newswise: Harvesting Light Like Nature Does
Released: 14-May-2021 2:55 PM EDT
Harvesting Light Like Nature Does
Pacific Northwest National Laboratory

A new class of bio-inspired two-dimensional (2D) hybrid nanomaterials mimic the ability of photosynthetic plants and bacteria.

Newswise: 050721-ber-earths-atomosphere.jpg?itok=-W-tcpvH
Released: 14-May-2021 2:50 PM EDT
Scientists Check the Math for Improved Models of Liquids and Gases in Earth’s Atmosphere
Department of Energy, Office of Science

Discretization is the process of converting continuous models and variables, such as wind speed, into discrete versions to make equations that are compatible with computer analysis. Energy consistent discretization ensures that the method does not have any inaccurate sources of energy that can lead to unstable and unrealistic simulations. In this research, scientists provided a discretization for equations used by global models of the Earth’s atmosphere.

View More

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